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Please use this identifier to cite or link to this item: https://dspace.iiti.ac.in/handle/123456789/16869
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dc.contributor.authorSrivastava, Navdeepen_US
dc.date.accessioned2025-09-23T12:04:34Z-
dc.date.available2025-09-23T12:04:34Z-
dc.date.issued2026-
dc.identifier.citationChoudhary, N., Srivastava, N., Annadata, H. V., Ghosh, B., & da Costa, P. (2026). Strategic integration of yttrium single atoms on CeO2 supported nickel catalysts for enhanced CO2 methanation catalysis. Applied Catalysis B: Environmental, 382. https://doi.org/10.1016/j.apcatb.2025.125918en_US
dc.identifier.issn0926-3373-
dc.identifier.otherEID(2-s2.0-105015373263)-
dc.identifier.urihttps://dx.doi.org/10.1016/j.apcatb.2025.125918-
dc.identifier.urihttps://dspace.iiti.ac.in:8080/jspui/handle/123456789/16869-
dc.description.abstractWe report the synthesis of a high-performance CO<inf>2</inf> methanation catalyst, Ni-Y<inf>1</inf>/CeO<inf>2</inf>, comprising Ni nanoparticles and atomically dispersed Y3 + on a ceria support. This precisely designed catalyst achieved an outstanding CO<inf>2</inf> conversion of 83 % with 100 % CH<inf>4</inf> selectivity at 350 °C. XAS unambiguously confirmed the atomic dispersion of Y3+ with the absence of any Y-Y bonds, while STEM-EDS revealed uniform Y distribution with finely dispersed Ni NPs. Enhanced oxygen vacancies and improved basic sites contributed to the superior activity of Ni-Y<inf>1</inf>/CeO<inf>2</inf> even at low temperature (250–300 °C) and showed excellent stability over 40 h. Comparative studies with impregnated NiY/CeO<inf>2</inf>-imp and Ni/CeO<inf>2</inf> highlighted the synergistic effect of Y3+ and Ni. These results establish Y3+ single-atom modulation as a powerful approach to tailoring basic sites and enhanced oxygen vacancies, unlocking new design pathways for advanced CO<inf>2</inf> methanation catalysts. © 2025 Elsevier B.V., All rights reserved.en_US
dc.language.isoenen_US
dc.publisherElsevier B.V.en_US
dc.sourceApplied Catalysis B: Environmentalen_US
dc.subjectCo2 Utilization And Recyclingen_US
dc.subjectInterfacial Sitesen_US
dc.subjectMethanationen_US
dc.subjectOxygen Vacancyen_US
dc.subjectSingle Atom Catalystsen_US
dc.subjectAtomsen_US
dc.subjectBinary Alloysen_US
dc.subjectCatalysisen_US
dc.subjectCatalyst Selectivityen_US
dc.subjectCatalyst Supportsen_US
dc.subjectCerium Oxideen_US
dc.subjectNickelen_US
dc.subjectNickel Compoundsen_US
dc.subjectSynthesis (chemical)en_US
dc.subjectTemperatureen_US
dc.subjectYttriumen_US
dc.subjectYttrium Compoundsen_US
dc.subjectBasic Sitesen_US
dc.subjectCatalyseen_US
dc.subjectCeo 2en_US
dc.subjectCo2 Utilization And Recyclingen_US
dc.subjectInterfacial Sitesen_US
dc.subjectSingle Atom Catalysten_US
dc.subjectSingle-atomsen_US
dc.subjectStrategic Integrationen_US
dc.subjectSupported Nickel Catalystsen_US
dc.subject]+ Catalysten_US
dc.subjectMethanationen_US
dc.subjectOxygen Vacanciesen_US
dc.titleStrategic integration of yttrium single atoms on CeO2 supported nickel catalysts for enhanced CO2 methanation catalysisen_US
dc.typeJournal Articleen_US
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